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    Intramolecular diffusive motion in alkane monolayers studied by high-resolution Quasielastic Neutron scattering and molecular dynamics simulations

    Hansen, Flemming Y.
    Criswell, Leah, 1971-
    Fuhrmann, D.
    Herwig, K. W.
    Diama, Armand, 1965-
    Dimeo, R. M.
    Neumann, Dan A.
    Volkmann, Ulrich G.
    Taub, Haskell
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    [PDF] IntramolecularDiffusiveMotionAlkane.pdf (244.4Kb)
    Date
    2004
    Format
    Article
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    Abstract
    Molecular dynamics simulations of a tetracosane (n-C24H50) monolayer adsorbed on a graphite basal-plane surface show that there are diffusive motions associated with the creation and annihilation of gauche defects occurring on a time scale of ~0.1-4 ns. We present evidence that these relatively slow motions are observable by high-energy-resolution quasielastic neutron scattering (QNS) thus demonstrating QNS as a technique, complementary to nuclear magnetic resonance, for studying conformational dynamics on a nanosecond time scale in molecular monolayers.
    URI
    http://hdl.handle.net/10355/8762
    Part of
    Missouri Research Reactor publications (MU)
    Citation
    Phys. Rev. Lett. 92, 046103 (2004)
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    • Missouri Research Reactor publications (MU)
    • Physics and Astronomy publications (MU)

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